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20210530151334.7 |
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210315s2021 gw a ob 001 0 eng d |
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|a 9783527825073
|q (electronic bk. : oBook)
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|a 352782507X
|q (electronic bk. : oBook)
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|a 9783527825097
|q electronic book
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|a 3527825096
|q electronic book
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|z 3527347186
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|z 9783527347186
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|a (NhCcYBP)ebc6516143
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|a NhCcYBP
|c NhCcYBP
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|a TJ810
|b .S65 2021
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|a 621.31/24
|2 23
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|a Solar-to-chemical conversion :
|b photocatalytic and photoelectrochemcial processes /
|c edited by Hongqi Sun.
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|a Weinheim, Germany :
|b Wiley-VCH,
|c [2021]
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|a 1 online resource.
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|a text
|b txt
|2 rdacontent
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|a computer
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|2 rdamedia
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|a online resource
|b cr
|2 rdacarrier
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|a Includes bibliographical references and index.
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|a Machine generated contents note:
|g 1.
|t Introduction: A Delicate Collection of Advances in Solar-to-Chemical Conversions /
|r Hongqi Sun --
|g 2.
|t Artificial Photosynthesis and Solar Fuels /
|r Jun Ke --
|g 2.1.
|t Introduction of Solar Fuels --
|g 2.2.
|t Photosynthesis --
|g 2.2.1.
|t Natural Photosynthesis --
|g 2.2.2.
|t Artificial Photosynthesis --
|g 2.3.
|t Principles of Photocatalysis --
|g 2.4.
|t Products of Artificial Photosynthesis --
|g 2.4.1.
|t Hydrocarbons --
|g 2.4.1.1.
|t Methane (CH4) --
|g 2.4.1.2.
|t Methanol (CH3OH) --
|g 2.4.1.3.
|t Formaldehyde (HCHO) --
|g 2.4.1.4.
|t Formic Acid (HCOOH) --
|g 2.4.1.5.
|t C2 Hydrocarbons --
|g 2.4.1.6.
|t Other Hydrocarbons --
|g 2.4.2.
|t Carbon Monoxide (CO) --
|g 2.4.3.
|t Dioxygen (O2) --
|g 2.5.
|t Perspective --
|t Acknowledgments --
|t References --
|g 3.
|t Natural and Artificial Photosynthesis /
|r Dimitrios A. Pantazis --
|g 3.1.
|t Introduction --
|g 3.2.
|t Overview of Natural Photosynthesis --
|g 3.3.
|t Light Harvesting and Excitation Energy Transfer --
|g 3.4.
|t Charge Separation and Electron Transfer --
|g 3.5.
|t Water Oxidation --
|g 3.6.
|t Carbon Fixation --
|g 3.7.
|t Conclusions --
|t References --
|g 4.
|t Photocatalytic Hydrogen Evolution /
|r Yijiao Jiang --
|g 4.1.
|t Introduction --
|g 4.2.
|t Fundamentals of Photocatalytic H2 Evolution --
|g 4.3.
|t Photocatalytic H2 Evolution Under UV Light --
|g 4.3.1.
|t Titanium Dioxide (TiO2)-Based Semiconductors --
|g 4.3.2.
|t Other Types of UV-Responsive Photocatalysts --
|g 4.4.
|t Photocatalytic H2 Evolution Under Visible Light --
|g 4.4.1.
|t Carbon Nitride (C3N4)-Based Semiconductor --
|g 4.4.2.
|t Other Types of Visible-Light-Responsive Photocatalysts --
|g 4.5.
|t Photocatalytic H2 Evolution Under Near-Infrared Light --
|g 4.6.
|t Roles of Sacrificial Reagents and Reaction Pathways --
|g 4.7.
|t Summary and Outlook --
|t References --
|g 5.
|t Photoelectrochemical Hydrogen Evolution /
|r Lianzhou Wang --
|g 5.1.
|t Background of Photoelectrocatalytic Water Splitting --
|g 5.2.
|t Mechanism of Charge Separation and Transfer --
|g 5.3.
|t Strategy for Improving Charge Transfer --
|g 5.3.1.
|t Improving the Charge Transfer in Continuous Film --
|g 5.3.2.
|t Improving the Charge Transfer in Particulate Photoelectrodes --
|g 5.4.
|t Strategy for Improving Electron-Hole Separation --
|g 5.4.1.
|t Heterojunction Formation --
|g 5.4.2.
|t Crystal Facet Control --
|g 5.4.3.
|t Surface Passivation --
|g 5.5.
|t Surface Cocatalyst Design --
|g 5.6.
|t Unbiased PEC Water Splitting --
|g 5.7.
|t Conclusion and Perspective --
|t References --
|g 6.
|t Photocatalytic Oxygen Evolution /
|r Shaobin Wang --
|g 6.1.
|t Introduction --
|g 6.1.1.
|t Configuration of Photocatalytic Water Oxidation --
|g 6.1.2.
|t Mechanism, Thermodynamics, and Kinetics Toward Efficient Oxygen Evolution --
|g 6.2.
|t Homogeneous Photocatalytic Water Oxidation --
|g 6.2.1.
|t Molecular Complexes and Polyoxometalates --
|g 6.2.2.
|t Mechanism Details and the Stability --
|g 6.3.
|t Heterogeneous Photocatalytic Water Oxidation --
|g 6.3.1.
|t Unique Properties of Nanosized Semiconductor System --
|g 6.3.1.1.
|t Quantum Confinement --
|g 6.3.1.2.
|t Localized Surface Plasmon Resonance (LSPR) --
|g 6.3.1.3.
|t Surface Area and Exposed Facet-Enhanced Charge Transfer --
|g 6.3.2.
|t Zero-Dimensional Semiconductor Materials for Photocatalytic Water Oxidation --
|g 6.3.2.1.
|t OD Metal Complexes and Nanoclusters --
|g 6.3.2.2.
|t Metal Oxide Quantum Dots and Nanocrystals --
|g 6.3.3.
|t One-Dimensional Semiconductor Materials for Photocatalytic Water Oxidation --
|g 6.3.4.
|t Two-Dimensional Semiconductor Materials for Photocatalytic Water Oxidation --
|g 6.3.4.1.
|t 2D Metal Oxide Nanosheets for Photocatalytic Water Oxidation --
|g 6.3.4.2.
|t Layered Double Hydroxide (LDH) Nanosheets for Photocatalytic Water Oxidation --
|g 6.3.4.3.
|t Metal-Based Oxyhalide Semiconductors for Photocatalytic Water Oxidation --
|g 6.3.5.
|t LD Semiconductor-Based Hybrids for Photocatalytic Oxygen Evolution --
|g 6.3.5.1.
|t ID-Based (0D/1D and 1D/1D) Semiconductor Hybrids for Enhanced Photocatalytic Water Oxidation --
|g 6.3.5.2.
|t 2D-Based (2D/2D) Semiconductor Hybrids for Enhanced Photocatalytic Water Oxidation --
|g 6.3.5.3.
|t Metal-Free-Based Semiconductors for Water Oxidation --
|g 6.4.
|t Catalytic Active Site-Catalysis Correlation in LD Semiconductors --
|g 6.5.
|t Conclusions and Perspectives --
|t References --
|g 7.
|t Photoelectrochemical Oxygen Evolution /
|r Fumiaki Amano --
|g 7.1.
|t Introduction --
|g 7.2.
|t Honda-Fujishima Effect --
|g 7.3.
|t Factors Affecting the Photoanodic Current --
|g 7.4.
|t Electrode Potentials at Different pH --
|g 7.5.
|t Evaluation of PEC Performance --
|g 7.6.
|t Flat Band Potential and Photocurrent Onset Potential --
|g 1.1.
|t Selection of Materials --
|g 7.8.
|t Enhancement of PEC Properties --
|g 7.8.1.
|t Nanostructuring and Morphology Control --
|g 7.8.2.
|t Donor Doping --
|g 7.8.3.
|t Modification of Photoanode Surface --
|g 7.8.4.
|t Electron-Conductive Materials --
|g 7.9.
|t PEC Device for Water Splitting --
|g 7.10.
|t Conclusions and Outlook --
|t References --
|g 8.
|t Photocatalytic and Photoelectrochemical Overall Water Splitting /
|r Dong Ha Kim --
|g 8.1.
|t Introduction --
|g 8.2.
|t Photocatalytic Overall Water Splitting --
|g 8.2.1.
|t Principles and Mechanism --
|g 8.2.2.
|t Key Performance Indicators --
|g 8.2.3.
|t Materials for One-Step Photoexcitation Toward Overall Water Splitting --
|g 8.2.3.1.
|t Semiconductors --
|g 8.2.3.2.
|t Incorporation of Cocatalysts --
|g 8.2.3.3.
|t Plasmonic Nanostructures --
|g 8.2.4.
|t Hybrid Systems for Two-Step Photoexcitation Toward Overall Water Splitting --
|g 8.2.4.1.
|t Z-Schemes --
|g 8.3.
|t Photoelectrochemical Overall Water Splitting --
|g 8.3.1.
|t Principles and Mechanism --
|g 8.3.2.
|t Key Performance Indicators --
|g 8.3.3.
|t Materials Design --
|g 8.3.3.1.
|t Photoanode Materials --
|g 8.3.3.2.
|t Photocathode Materials --
|g 8.3.4.
|t Unassisted Photoelectrochemical Overall Water Splitting --
|g 8.3.4.1.
|t Photoanode-Photocathode Tandem Cells --
|g 8.3.4.2.
|t Photovoltaic-Photoelectrode Devices --
|g 8.4.
|t Concluding Remarks and Outlook --
|t Acknowledgments --
|t References --
|g 9.
|t Photocatalytic CO2 Reduction /
|r Qibin Liu --
|g 9.1.
|t Introduction --
|g 9.2.
|t Principle of Photocatalytic Reduction of C02 --
|g 9.3.
|t Energy and Mass Transfers in Photocatalytic Reduction of C02 --
|g 9.3.1.
|t Energy Flow from the Concentrator to Reactor --
|g 9.3.2.
|t Energy Flow on the Surface of the Photocatalyst --
|g 9.3.3.
|t Mass Flow in C02 Photocatalytic Reduction --
|g 9.3.4.
|t Product Selectivity in C02 Photocatalytic Reaction --
|g 9.4.
|t Conclusions --
|t Acknowledgments --
|t References --
|g 10.
|t Photoelectrochemical C02 Reduction /
|r Mingbo Wu --
|g 10.1.
|t Introduction --
|g 10.1.1.
|t Introduction of Photoelectrocatalytic Reduction of CO2 --
|g 10.1.2.
|t Principles of Photoelectrocatalytic Reduction of CO2 --
|g 10.1.3.
|t System Configurations of Photoelectrocatalytic Reduction ofC02 --
|g 10.2.
|t PEC CO2 Reduction Principles --
|g 10.2.1.
|t Thermodynamics and Kinetics of CO2 Reduction --
|g 10.2.2.
|t Reaction Conditions --
|g 10.2.2.1.
|t Reaction Temperature and Pressure --
|g 10.2.2.2.
|t Ph Value --
|g 10.2.2.3.
|t Solvent --
|g 10.2.2.4.
|t External Electrical Bias --
|g 10.2.3.
|t Performance Evaluation of PEC CO2 Reduction --
|g 10.2.3.1.
|t Product Evolution Rate and Catalytic Current Density --
|g 10.2.3.2.
|t Turnover Number and Turnover Frequency --
|g 10.2.3.3.
|t Overpotential --
|g 10.2.3.4.
|t Faradaic Efficiency --
|g 10.3.
|t Application of Solar-to-Chemical Energy Conversion in PEC CO2 Reduction --
|g 10.3.1.
|t PEC C02 Reduction on Semiconductors --
|g 10.3.1.1.
|t Oxide Semiconductors --
|g 10.3.1.2.
|t Non-oxide Semiconductors --
|g 10.3.1.3.
|t Chalcogenide Semiconductors --
|g 10.3.2.
|t PEC C02 Reduction on Cocatalyst Systems --
|g 10.3.2.1.
|t Metal Nanoparticles --
|g 10.3.2.2.
|t Metal Complexes --
|g 10.3.3.
|t PEC C02 Reduction on Hybrid Semiconductors --
|g 10.3.3.1.
|t Conductive Polymers --
|g 10.3.3.2.
|t Enzymatic Biocatalysts --
|g 10.3.3.3.
|t Organic Molecules --
|g 10.4.
|t Other Configurations for PEC CO2 Reduction --
|g 10.5.
|t Conclusion and Outlook --
|t Acknowledgments --
|t Conflict of Interest --
|t References --
|g 11.
|t Photocatalytic and Photoelectrochemical Nitrogen Fixation /
|r Hongqi Sun --
|g 11.1.
|t Introduction --
|g 11.2.
|t Fundamental Principles and Present Challenges --
|g 11.2.1.
|t Principles in N2 Reduction for NH3 Production --
|g 11.2.2.
|t Challenges for N2 Reduction to NH3 --
|g 11.3.
|t Strategies for Catalyst Design and Fabrication --
|g 11.3.1.
|t Defect Engineering --
|g 11.3.1.1.
|t Vacancies --
|g 11.3.1.2.
|t Heteroatom Doping --
|g 11.3.1.3.
|t Amorphization --
|g 11.3.2.
|t Structure Engineering --
|g 11.3.2.1.
|t Morphology Regulation --
|g 11.3.2.2.
|t Facet Control --
|g 11.3.3.
|t Interface Engineering --
|g 11.3.4.
|t Heterojunction Engineering --
|g 11.3.5.
|t Co-catalyst Engineering --
|g 11.3.6.
|t Biomimetic Engineering --
|g 11.4.
|t Conclusions and Outlook --
|t References --
|g 12.
|t Photocatalytic Production of Hydrogen Peroxide Using MOF Materials /
|r Hiromi Yamashita --
|g 12.1.
|t Introduction --
|g 12.2.
|t Photocatalytic H2O2 Production Through Selective Two-Electron Reduction of O2 Utilizing NiO/MIL-125-NH2 --
|g 12.3.
|t Two-Phase System Utilizing Linker-Alkylated Hydrophobic MIL-125-NH2 for Photocatalytic H2O2 Production --
|g 12.4.
|t Ti Cluster-Alkylated Hydrophobic MIL-125-NH, for Photocatalytic H2O2 Production in Two-Phase System --
|g 12.5.
|t Conclusion and Outlooks --
|t Reference --
|g 13.
|t Photocatalytic and Photoelectrochemical Reforming of Methane /
|r Hongqi Sun --
|g 13.1.
|t Introduction --
|g 13.2.
|t Photo-Mediated Processes --
|g 13.3.
|t Differences Between Photo-Assisted Catalysis and Thermocatalysis --
|g 13.3.1.
|t Catalyst Involved --
|g 13.3.2.
|t Reactors --
|g 13.3.3.
|t Mechanism --
|g 13.3.4.
|t Equations for Quantum Efficiency --
|g 13.4.
|t Reactions of Methane Conversion via Photo-Assisted Catalysis --
|g 13.4.1.
|t Methane Dry Reforming --
|g 13.4.2.
|t Methane Steam Reforming --
|g 13.4.3.
|t Methane Coupling --
|g 13.4.4.
|t Methane Oxidation --
|g 13.4.5.
|t Methane Dehydroaromatization --
|g 13.5.
|t Conclusions and Perspectives --
|t Acknowledgment --
|t References --
|
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|a Contents note continued:
|g 14.
|t Photocatalytic and Photoelectrochemical Reforming of Biomass /
|r Bing-Jie Ni --
|g 14.1.
|t Introduction --
|g 14.2.
|t Fundamentals of Photocatalytic and Photoelectrochemical Processes --
|g 14.2.1.
|t Photocatalytic Process --
|g 14.2.2.
|t Photoelectrochemical Process --
|g 14.3.
|t Photocatalytic Reforming of Biomass --
|g 14.3.1.
|t Photocatalytic Reforming of Lignin --
|g 14.3.2.
|t Photocatalytic Reforming of Carbohydrates --
|g 14.3.3.
|t Photocatalytic Reforming of Native Lignocellulose --
|g 14.3.4.
|t Photocatalytic Reforming of Triglycerides and Glycerol --
|g 14.4.
|t Photoelectrochemical Reforming of Biomass --
|g 14.4.1.
|t Photoelectrochemical Conversion of Biomass to Produce Electricity --
|g 14.4.2.
|t Photoelectrochemical Conversion of Biomass to Produce Hydrogen --
|g 14.4.3.
|t Photoelectrochemical Conversion of Biomass to Produce Chemicals --
|g 14.5.
|t Conclusion Remarks and Perspectives --
|t Acknowledgments --
|t References --
|g 15.
|t Reactors, Fundamentals, and Engineering Aspects for Photocatalytic and Photoelectrochemical Systems /
|r Siang-Piao Chai --
|g 15.1.
|t Fundamental Mechanisms of Photocatalytic and PEC Processes --
|g 15.1.1.
|t Rationales of Photocatalytic Systems --
|g 15.1.1.1.
|t Photocatalytic Water Splitting --
|g 15.1.1.2.
|t Photocatalytic CO2 reduction --
|g 15.1.2.
|t Rationales of PEC Systems --
|g 15.2.
|t Reactor Design and Configuration --
|g 15.2.1.
|t Reactors for Photocatalytic Systems --
|g 15.2.1.1.
|t Reactors for Photocatalytic Water Splitting --
|g 15.2.1.2.
|t Reactors for Photocatalytic CO2 Reduction --
|g 15.2.2.
|t Reactors for PEC Systems --
|g 15.3.
|t Engineering Aspects of Photocatalytic and PEC Processes --
|g 15.3.1.
|t Photocatalyst Sheets: Scaling-up of Photocatalytic Water Splitting --
|g 15.3.2.
|t Monolithic Devices: Wireless Approach of PEC Reaction --
|g 15.4.
|t Conclusions and Outlook --
|t Acknowledgments --
|t List of Abbreviations --
|t References --
|g 16.
|t Prospects of Solar Fuels /
|r Hongqi Sun.
|
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|a Electronic reproduction.
|b Ann Arbor, MI
|n Available via World Wide Web.
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|a Description based on online resource; title from digital title page (viewed on April 27, 2021).
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|a Solar energy.
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|a Energy conversion.
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|a Sun, Hongqi,
|e editor.
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|a ProQuest (Firm)
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